I use the vocab and definitions almost exactly as Croy does.
I prefer to learn a noun with its article. This way, when you're recalling it, you'll always have the gender of it memorized.
I also like to learn prepositions, their cases, and their meaning separately.
i.e. περί (+ gen.) = about, concerning
περί (+ acc.) = around
This is the way I have found most useful. If you're not a fan, you can create your own lists perfectly customized to your needs.
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